表面等离激元与激子的强耦合作用

doi:10.13190/j.jbupt.2021-257

北京邮电大学学报 ›› 2022, Vol. 45 ›› Issue (3): 7-12.doi: 10.13190/j.jbupt.2021-257

表面等离激元与激子的强耦合作用

梁琨¹, 于丽²

1. 北京邮电大学电子工程学院, 北京 100876;
2. 北京邮电大学理学院, 北京 100876

收稿日期:2021-11-02 出版日期:2022-06-28 发布日期:2022-06-01
通讯作者: 于丽(1963—),女,教授,邮箱:yuliyuli@bupt.edu.cn。 E-mail:yuliyuli@bupt.edu.cn
作者简介:梁琨(1992—),男,博士后。
基金资助:
国家自然基金面上项目(12174037)

Strong Coupling Between Surface Plasmons and Excitons

LIANG Kun¹, YU Li²

1. School of Electronic Engineering, Beijing University of Posts and Telecommunications, Beijing 100876, China;
2. School of Science, Beijing University of Posts and Telecommunications, Beijing 100876, China

Received:2021-11-02 Online:2022-06-28 Published:2022-06-01

摘要/Abstract

摘要： 金属纳米结构中高度局域的表面等离激元模式给光与物质的强相互作用带来了新的研究机遇。在特定条件下,二者的相干能量交换速率会超越各自的能量耗散速率,进入强耦合范畴,该过程可形成光子-激子杂化的准粒子。针对近年来飞速发展的量子光学调控,特别是基于表面等离激元体系的强耦合研究展开综述,介绍了如金属纳腔与手性J聚体强耦合,在零失谐点对耦合系统进行精细调控,通过微流技术实现可控的表面等离激元纳腔-少激子强耦合等。在亚波长尺度下研究强耦合系统中的光场调控技术,有助于光电子器件的小型化。强耦合体系在片上集成的量子信息处理、手性光学器件和超灵敏生化传感器等领域有广阔的应用前景。

关键词: 局域表面等离激元, 激子, 手性, 强耦合, 调控

Abstract: The condensed electromagnetic field of localized surface plasmon mode in metallic nanocavities brought new opportunities in studying the strong light-matter interaction. Under certain conditions, the rate of coherent energy exchange between a cavity photon and an electronic transition surpasses its fundamental energy dissipation rates, which is defined as the strong coupling regime. This process may generate a part-light part-matter quasi-particle, which is known as a hybrid polariton. A series of recent works in quantum optics is summarized, particularly on studying the strong coupling phenomenon and its dynamic control in plasmonic systems, such as strong coupling between metallic nanocavities and chiral J-aggregates, fine-tuning of polariton energies near zero-detuned point, and active control of excitons strongly coupled to plasmonic nano-cavities using a microfluidic technique. Exploring the active control of the optical field on a sub-wavelength scale is valuable, which benefits the miniaturization of optoelectronic devices. Strong coupling systems possess wide application prospects, such as quantum information processing and ultra-sensitive biochemical detections.

Key words: localized surface plasmon polaritons, excitons, chirality, strong coupling, active control

中图分类号:

O431.2

梁琨, 于丽. 表面等离激元与激子的强耦合作用[J]. 北京邮电大学学报, 2022, 45(3): 7-12.

LIANG Kun, YU Li. Strong Coupling Between Surface Plasmons and Excitons[J]. Journal of Beijing University of Posts and Telecommunications, 2022, 45(3): 7-12.

参考文献

[1] WANG S, WANG X Y, LI B, et al. Unusual scaling laws for plasmonic nano-lasers beyond the diffraction limit[J]. Nature Communications, 2017, 8(1):1-8.
[2] KOYA A N, CUNHA J, GUO T L, et al. Novel plasmonic nanocavities for optical trapping-assisted biosensing applications[J]. Advanced Optical Materials, 2020, 8(7):1901481-1901492.
[3] JIANG X H, CHEN P, QIAN K Y, et al. Quantum teleportation mediated by surface plasmon polariton[J]. Scientific Reports, 2020, 10(1):1-8.
[4] TIECKE T, THOMPSON J D, LEON N P, et al. Nanophotonic quantum phase switch with a single atom[J]. Nature, 2014, 508(7495):241-244.
[5] WEI H, YAN X, NIU Y, et al. Plasmon-exciton interactions:spontaneous emission and strong coupling[J]. Advanced Functional Materials, 2021, 31(51):2100889-2100907.
[6] DING D, PEREIRA L M, BAUTERS J F, et al. Multidimensional Purcell effect in an ytterbium-doped ring resonator[J]. Nature Photonics, 2016, 10(6):385-388.
[7] GALFSKY T, SUN Z, CONSIDINE C R, et al. Broadband enhancement of spontaneous emission in two-dimensional semiconductors using photonic hyper-crystals[J]. Nano Letters, 2016, 16(8):4940-4045.
[8] 周张凯,李俊韬,刘仁明,等.固态光学微腔与量子体系相互耦合的调控及其量子器件研究[J].中国基础科学, 2019, 21(6):12-20. ZHOU Z K, LI J T, LIU R M, et al. Investigations on the coupling manipulation and device application in the compound system of solid optical microcavity and quantum system[J]. China Basic Science, 2019, 21(6):12-20.
[9] BAUMANN K, GUERLIN C, BRENNECKE F, et al. Dicke quantum phase transition with a superfluid gas in an optical cavity[J]. Nature, 2010, 464(7293):1301-1306.
[10] MOILANEN A J, HAKALA T K, TÖRMÄ P. Active control of surface plasmon-emitter strong coupling[J]. ACS Photonics, 2018, 5(1):54-64.
[11] LODAHL P, MAHMOODIAN S, STOBBE S, et al. Chiral quantum optics[J]. Nature, 2017, 541(7638):473-480.
[12] ZHENG D, ZHANG S, DENG Q, et al. Manipulating coherent plasmon-exciton interaction in a single silver nanorod on monolayer WSe2[J]. Nano Letters, 2017, 17(6):3809-3814.
[13] HUANG Y, WANG Y, LIANG K, et al. Quantum theory of nonradiative decay dependent on the coupling strength in a plexcitonic system[J]. Optical Express, 2021, 29(26):43292-43303.
[14] REMPE G, WALTHER H, KLEIN N. Observation of quantum collapse and revival in a one-atom maser[J]. Physical Review Letters, 1987, 58(4):353-362.
[15] REITHMAIER J P, SęK G, LÖFFLER A, et al. Strong coupling in a single quantum dot-semiconductor microcavity system[J]. Nature, 2004, 432(7014):197-200.
[16] ARMANI D, KIPPENBERG T, SPILLANE S, et al. Ultra-high toroid microcavity on a chip[J]. Nature, 2003, 421(6926):925-928.
[17] POCKRAND I, BRILLANTE A, MÖBIUS D. Exciton-surface plasmon coupling:an experimental investigation[J]. The Journal of Chemical Physics, 1982, 77(12):6289-6295.
[18] HOBSON P A, BARNES W L, LIDZEY D, et al. Strong exciton-photon coupling in a low-Q all-metal mirror microcavity[J]. Applied Physics Letters, 2002, 81(19):3519-3521.
[19] SCHWARTZ T, HUTCHISON J A, GENET C, et al. Reversible switching of ultra-strong light-molecule coupling[J]. Physical Review Letters, 2011, 106(19):196405-196409.
[20] VASA P, WANG W, POMRAENKE R, et al. Real-time observation of ultrafast Rabi oscillations between excitons and plasmons in metal nanostructures with J-aggregates[J]. Nature Photonics, 2013, 7(2):128-132.
[21] KRAVETS V G, KABASHIN A V, BARNES W L, et al. Plasmonic surface lattice resonances:a review of properties and applications[J]. Chemical Reviews, 2018, 118(12):5912-5951.
[22] KRAVETS V G, KABASHIN A V, BARNES W L, et al. Plasmonic surface lattice resonances:a review of properties and applications[J]. Chemical Reviews, 2018, 118(12):5912-5951.
[23] SCHLATHER A E, LARGE N, URBAN A S, et al. Near-field mediated pl-excitonic coupling and giant Rabi splitting in individual metallic dimers[J]. Nano Letters, 2013, 13(7):3281-3286.
[24] LIANG K, GUO J, HUANG Y, et al. Fine-tuning of polariton energies in a tailored plasmon cavity and J-aggregates hybrid system[J]. Nanoscale, 2020, 12(45):23069-23076.
[25] HENSEN M, HEILPERN T, GRAY S K, et al. Strong coupling and entanglement of quantum emitters embedded in a nanoantenna-enhanced plasmonic cavity[J]. ACS Photonics, 2018, 5(1):240-248.
[26] LIANG K, GUO J, WU F, et al. Dynamic control of quantum emitters strongly coupled to the isolated plasmon cavity by the microfluidic device[J]. The Journal of Physical Chemistry C, 2021, 125(31):17303-17310.
[27] FRANKS M E, MACPHERSON G R, FIGG W D. Thalidomide[J]. The Lancet, 2004, 363(9423):1802-1811.
[28] SONG L, GUO Z, CHEN Y. Separation and determination of chiral composition in penicillamine tablets by capillary electrophoresis in a broad pH range[J]. Electrophoresis, 2012, 33(13):2056-2063.
[29] SLOCIK J M, GOVOROV A O, NAIK R R. Plasmonic circular dichroism of peptide-functionalized gold nano-particles[J]. Nano Letters, 2011, 11(2):701-705.
[30] SHEN Z, JIANG Y, WANG T, et al. Symmetry brea-king in the supramolecular gels of an achiral gelator exclusively driven by π-π stacking[J]. Journal of the American Chemical Society, 2015, 137(51):16109-16115.
[31] GUAN A J, ZHANG J T, WANG L X, et al. Sponta-neous formation and reversible transformation between achiral J-and chiral H-aggregates of cyanine dye MTC[J]. RSC Advances, 2019, 9(20):11365-11368.
[32] GUO J, SONG G, HUANG Y, et al. Optical chirality in a strong coupling system with surface plasmons polaritons and chiral emitters[J]. ACS Photonics, 2021, 8(3):901-906.
[33] WU F, GUO J, HUANG Y, et al. Plexcitonic optical chirality:strong exciton-plasmon coupling in chiral J-aggregate-metal nanoparticle complexes[J]. ACS Nano, 2020, 15(2):2292-2300.

表面等离激元与激子的强耦合作用

Strong Coupling Between Surface Plasmons and Excitons

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